Electrochemiluminescent swimmers for dynamic enzymatic sensing
Само за регистроване кориснике
2014
Аутори
Sentić, MilicaArbault, Stephane
Goudeau, Bertrand
Manojlović, Dragan D.
Kuhn, Alexander
Bouffier, Laurent
Šojić, Nešo
Чланак у часопису (Објављена верзија)
Метаподаци
Приказ свих података о документуАпстракт
An electrochemiluminescent (ECL) swimmer driven by bipolar electrochemistry is reported for enzymatic glucose sensing. The chemomechanical motion is induced by localized hydrogen bubble generation. The concomitant oxidation of the luminophore and of the enzymatically-produced NADH leads to ECL emission with a direct glucose-dependent light intensity. We demonstrate herein the local sensing and reporting of glucose in a concentration gradient explored by the ECL swimmer. Such a dynamic sensing approach combines in a synergetic way the wireless propulsion with the enzymatic selectivity using ECL as a readout method at the level of moving objects.
Извор:
Chemical Communications, 2014, 50, 71, 10202-10205Издавач:
- Royal Soc Chemistry, Cambridge
Финансирање / пројекти:
- French Foreign Ministry (Bourse dExcellence Eiffel)
- Ministry of Science and Technological Development (Republic of Serbia)
DOI: 10.1039/c4cc04105d
ISSN: 1359-7345
PubMed: 24999792
WoS: 000340896900004
Scopus: 2-s2.0-84905728128
Колекције
Институција/група
Hemijski fakultet / Faculty of ChemistryTY - JOUR AU - Sentić, Milica AU - Arbault, Stephane AU - Goudeau, Bertrand AU - Manojlović, Dragan D. AU - Kuhn, Alexander AU - Bouffier, Laurent AU - Šojić, Nešo PY - 2014 UR - https://cherry.chem.bg.ac.rs/handle/123456789/1834 AB - An electrochemiluminescent (ECL) swimmer driven by bipolar electrochemistry is reported for enzymatic glucose sensing. The chemomechanical motion is induced by localized hydrogen bubble generation. The concomitant oxidation of the luminophore and of the enzymatically-produced NADH leads to ECL emission with a direct glucose-dependent light intensity. We demonstrate herein the local sensing and reporting of glucose in a concentration gradient explored by the ECL swimmer. Such a dynamic sensing approach combines in a synergetic way the wireless propulsion with the enzymatic selectivity using ECL as a readout method at the level of moving objects. PB - Royal Soc Chemistry, Cambridge T2 - Chemical Communications T1 - Electrochemiluminescent swimmers for dynamic enzymatic sensing VL - 50 IS - 71 SP - 10202 EP - 10205 DO - 10.1039/c4cc04105d ER -
@article{ author = "Sentić, Milica and Arbault, Stephane and Goudeau, Bertrand and Manojlović, Dragan D. and Kuhn, Alexander and Bouffier, Laurent and Šojić, Nešo", year = "2014", abstract = "An electrochemiluminescent (ECL) swimmer driven by bipolar electrochemistry is reported for enzymatic glucose sensing. The chemomechanical motion is induced by localized hydrogen bubble generation. The concomitant oxidation of the luminophore and of the enzymatically-produced NADH leads to ECL emission with a direct glucose-dependent light intensity. We demonstrate herein the local sensing and reporting of glucose in a concentration gradient explored by the ECL swimmer. Such a dynamic sensing approach combines in a synergetic way the wireless propulsion with the enzymatic selectivity using ECL as a readout method at the level of moving objects.", publisher = "Royal Soc Chemistry, Cambridge", journal = "Chemical Communications", title = "Electrochemiluminescent swimmers for dynamic enzymatic sensing", volume = "50", number = "71", pages = "10202-10205", doi = "10.1039/c4cc04105d" }
Sentić, M., Arbault, S., Goudeau, B., Manojlović, D. D., Kuhn, A., Bouffier, L.,& Šojić, N.. (2014). Electrochemiluminescent swimmers for dynamic enzymatic sensing. in Chemical Communications Royal Soc Chemistry, Cambridge., 50(71), 10202-10205. https://doi.org/10.1039/c4cc04105d
Sentić M, Arbault S, Goudeau B, Manojlović DD, Kuhn A, Bouffier L, Šojić N. Electrochemiluminescent swimmers for dynamic enzymatic sensing. in Chemical Communications. 2014;50(71):10202-10205. doi:10.1039/c4cc04105d .
Sentić, Milica, Arbault, Stephane, Goudeau, Bertrand, Manojlović, Dragan D., Kuhn, Alexander, Bouffier, Laurent, Šojić, Nešo, "Electrochemiluminescent swimmers for dynamic enzymatic sensing" in Chemical Communications, 50, no. 71 (2014):10202-10205, https://doi.org/10.1039/c4cc04105d . .