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Degradation of nicotine in water solutions using a water falling film DBD plasma reactor: direct and indirect treatment

Authorized Users Only
2018
Authors
Krupež, Jelena
Kovačević, Vesna V.
Jović, Milica
Roglić, Goran
Natić, Maja
Kuraica, Milorad M.
Obradović, Bratislav M.
Dojčinović, Biljana P.
Article (Published version)
Metadata
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Abstract
Nicotine degradation efficiency in water solutions was studied using a water falling film dielectric barrier discharge (DBD) reactor. Two different treatments were applied: direct treatment, the recirculation of the solution through a DBD reactor, and indirect treatment, the bubbling of the gas from the DBD through the porous filter into the solution. In a separate experiment, samples spiked with nicotine in double distilled water (ddH(2)O) and tap water were studied and compared after both treatments. Furthermore, the effects of the homogeneous catalysts, namely, Fe2+ and H2O2, were tested in the direct treatment. Nicotine degradation efficiency was determined using high-performance liquid chromatography. A degradation efficiency of 90% was achieved after the direct treatment catalyzed with Fe2+. In order to analyze the biodegradability, mineralization level, and toxicity of the obtained solutions, after all degradation procedures the values of the following parameters were determined...: total organic carbon, chemical oxygen demand, biochemical oxygen demand, and the Artemia salina toxicity test. The results showed that an increase in biodegradability was obtained, after all treatments. A partial nicotine mineralization was achieved and the mortality of the A. salina organism decreased in the treated samples, all of which indicating the effective removal of nicotine and the creation of less toxic solutions. Nicotine degradation products were identified using ultrahigh-performance liquid chromatography coupled with a linear ion trap Orbitrap hybrid mass spectrometer and a simple mechanism for oxidative degradation of nicotine in non-thermal plasma systems is proposed.

Keywords:
advanced oxidation processes (AOP) / alkaloid / nicotine / wastewater treatment / water falling film DBD
Source:
Journal of Physics. D: Applied Physics, 2018, 51, 17
Publisher:
  • Iop Publishing Ltd, Bristol
Funding / projects:
  • Application of advanced oxidation processes and nanostructured oxide materials for the removal of pollutants from the environment, development and optimisation of instrumental techniques for efficiency monitoring (RS-172030)
  • Diagnostics and Optimization of Plasma Sources Important for Applications (RS-171034)
  • Integrated systems for flue gas cleansing and development of technologies for zero pollution power plants (RS-33022)

DOI: 10.1088/1361-6463/aab632

ISSN: 0022-3727

WoS: 000429231900001

Scopus: 2-s2.0-85045552718
[ Google Scholar ]
13
10
URI
https://cherry.chem.bg.ac.rs/handle/123456789/2126
Collections
  • Publikacije
Institution/Community
Hemijski fakultet
TY  - JOUR
AU  - Krupež, Jelena
AU  - Kovačević, Vesna V.
AU  - Jović, Milica
AU  - Roglić, Goran
AU  - Natić, Maja
AU  - Kuraica, Milorad M.
AU  - Obradović, Bratislav M.
AU  - Dojčinović, Biljana P.
PY  - 2018
UR  - https://cherry.chem.bg.ac.rs/handle/123456789/2126
AB  - Nicotine degradation efficiency in water solutions was studied using a water falling film dielectric barrier discharge (DBD) reactor. Two different treatments were applied: direct treatment, the recirculation of the solution through a DBD reactor, and indirect treatment, the bubbling of the gas from the DBD through the porous filter into the solution. In a separate experiment, samples spiked with nicotine in double distilled water (ddH(2)O) and tap water were studied and compared after both treatments. Furthermore, the effects of the homogeneous catalysts, namely, Fe2+ and H2O2, were tested in the direct treatment. Nicotine degradation efficiency was determined using high-performance liquid chromatography. A degradation efficiency of 90% was achieved after the direct treatment catalyzed with Fe2+. In order to analyze the biodegradability, mineralization level, and toxicity of the obtained solutions, after all degradation procedures the values of the following parameters were determined: total organic carbon, chemical oxygen demand, biochemical oxygen demand, and the Artemia salina toxicity test. The results showed that an increase in biodegradability was obtained, after all treatments. A partial nicotine mineralization was achieved and the mortality of the A. salina organism decreased in the treated samples, all of which indicating the effective removal of nicotine and the creation of less toxic solutions. Nicotine degradation products were identified using ultrahigh-performance liquid chromatography coupled with a linear ion trap Orbitrap hybrid mass spectrometer and a simple mechanism for oxidative degradation of nicotine in non-thermal plasma systems is proposed.
PB  - Iop Publishing Ltd, Bristol
T2  - Journal of Physics. D: Applied Physics
T1  - Degradation of nicotine in water solutions using a water falling film DBD plasma reactor: direct and indirect treatment
VL  - 51
IS  - 17
DO  - 10.1088/1361-6463/aab632
UR  - Kon_3457
ER  - 
@article{
author = "Krupež, Jelena and Kovačević, Vesna V. and Jović, Milica and Roglić, Goran and Natić, Maja and Kuraica, Milorad M. and Obradović, Bratislav M. and Dojčinović, Biljana P.",
year = "2018",
abstract = "Nicotine degradation efficiency in water solutions was studied using a water falling film dielectric barrier discharge (DBD) reactor. Two different treatments were applied: direct treatment, the recirculation of the solution through a DBD reactor, and indirect treatment, the bubbling of the gas from the DBD through the porous filter into the solution. In a separate experiment, samples spiked with nicotine in double distilled water (ddH(2)O) and tap water were studied and compared after both treatments. Furthermore, the effects of the homogeneous catalysts, namely, Fe2+ and H2O2, were tested in the direct treatment. Nicotine degradation efficiency was determined using high-performance liquid chromatography. A degradation efficiency of 90% was achieved after the direct treatment catalyzed with Fe2+. In order to analyze the biodegradability, mineralization level, and toxicity of the obtained solutions, after all degradation procedures the values of the following parameters were determined: total organic carbon, chemical oxygen demand, biochemical oxygen demand, and the Artemia salina toxicity test. The results showed that an increase in biodegradability was obtained, after all treatments. A partial nicotine mineralization was achieved and the mortality of the A. salina organism decreased in the treated samples, all of which indicating the effective removal of nicotine and the creation of less toxic solutions. Nicotine degradation products were identified using ultrahigh-performance liquid chromatography coupled with a linear ion trap Orbitrap hybrid mass spectrometer and a simple mechanism for oxidative degradation of nicotine in non-thermal plasma systems is proposed.",
publisher = "Iop Publishing Ltd, Bristol",
journal = "Journal of Physics. D: Applied Physics",
title = "Degradation of nicotine in water solutions using a water falling film DBD plasma reactor: direct and indirect treatment",
volume = "51",
number = "17",
doi = "10.1088/1361-6463/aab632",
url = "Kon_3457"
}
Krupež, J., Kovačević, V. V., Jović, M., Roglić, G., Natić, M., Kuraica, M. M., Obradović, B. M.,& Dojčinović, B. P.. (2018). Degradation of nicotine in water solutions using a water falling film DBD plasma reactor: direct and indirect treatment. in Journal of Physics. D: Applied Physics
Iop Publishing Ltd, Bristol., 51(17).
https://doi.org/10.1088/1361-6463/aab632
Kon_3457
Krupež J, Kovačević VV, Jović M, Roglić G, Natić M, Kuraica MM, Obradović BM, Dojčinović BP. Degradation of nicotine in water solutions using a water falling film DBD plasma reactor: direct and indirect treatment. in Journal of Physics. D: Applied Physics. 2018;51(17).
doi:10.1088/1361-6463/aab632
Kon_3457 .
Krupež, Jelena, Kovačević, Vesna V., Jović, Milica, Roglić, Goran, Natić, Maja, Kuraica, Milorad M., Obradović, Bratislav M., Dojčinović, Biljana P., "Degradation of nicotine in water solutions using a water falling film DBD plasma reactor: direct and indirect treatment" in Journal of Physics. D: Applied Physics, 51, no. 17 (2018),
https://doi.org/10.1088/1361-6463/aab632 .,
Kon_3457 .

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