Efficiency of Ni Nanoparticles Supported on Hierarchical Porous Nitrogen-Doped Carbon for Hydrogenolysis of Kraft Lignin in Flow and Batch Systems
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2017
Authors
Lama, Sandy M.G.Pampel, Jonas
Fellinger, Tim-Patrick
Beškoski, Vladimir
Slavković-Beškoski, Latinka
Antonietti, Markus
Molinari, Valerio
Article (Published version)
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Show full item recordAbstract
Ni nanoparticles supported on nitrogen-doped carbon (NDC) prepared via salt-melt synthesis with a hierarchical porosity were successfully applied as the catalyst for the degradation of Kraft lignin. It is shown that Ni-NDC is more efficient when compared to Ni nanoparticles deposited on an N-free carbon support, prepared with similar porosity features (Ni-C) and to Ni nanoparticles deposited on a commercial carbon (Ni-Cref). The efficiency of these materials was compared for reactions performed both in batch and flow reactors, highlighting the effect of the reactor setup on the stability of the recovered catalysts.
Keywords:
Kraft lignin / Heterogeneous catalysis / Nitrogen-doped carbon / Nickel / Hydrogenation / Porosity / Flow and batch system / Hierarchical porositySource:
ACS Sustainable Chemistry and Engineering, 2017, 5, 3, 2415-2420Publisher:
- Amer Chemical Soc, Washington
Funding / projects:
- Max Planck Institute
Note:
- Supplementary material: http://cherry.chem.bg.ac.rs/handle/123456789/3049
DOI: 10.1021/acssuschemeng.6b02761
ISSN: 2168-0485
WoS: 000395846900045
Scopus: 2-s2.0-85014533837
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Institution/Community
Hemijski fakultet / Faculty of ChemistryTY - JOUR AU - Lama, Sandy M.G. AU - Pampel, Jonas AU - Fellinger, Tim-Patrick AU - Beškoski, Vladimir AU - Slavković-Beškoski, Latinka AU - Antonietti, Markus AU - Molinari, Valerio PY - 2017 UR - https://cherry.chem.bg.ac.rs/handle/123456789/2427 AB - Ni nanoparticles supported on nitrogen-doped carbon (NDC) prepared via salt-melt synthesis with a hierarchical porosity were successfully applied as the catalyst for the degradation of Kraft lignin. It is shown that Ni-NDC is more efficient when compared to Ni nanoparticles deposited on an N-free carbon support, prepared with similar porosity features (Ni-C) and to Ni nanoparticles deposited on a commercial carbon (Ni-Cref). The efficiency of these materials was compared for reactions performed both in batch and flow reactors, highlighting the effect of the reactor setup on the stability of the recovered catalysts. PB - Amer Chemical Soc, Washington T2 - ACS Sustainable Chemistry and Engineering T1 - Efficiency of Ni Nanoparticles Supported on Hierarchical Porous Nitrogen-Doped Carbon for Hydrogenolysis of Kraft Lignin in Flow and Batch Systems VL - 5 IS - 3 SP - 2415 EP - 2420 DO - 10.1021/acssuschemeng.6b02761 ER -
@article{ author = "Lama, Sandy M.G. and Pampel, Jonas and Fellinger, Tim-Patrick and Beškoski, Vladimir and Slavković-Beškoski, Latinka and Antonietti, Markus and Molinari, Valerio", year = "2017", abstract = "Ni nanoparticles supported on nitrogen-doped carbon (NDC) prepared via salt-melt synthesis with a hierarchical porosity were successfully applied as the catalyst for the degradation of Kraft lignin. It is shown that Ni-NDC is more efficient when compared to Ni nanoparticles deposited on an N-free carbon support, prepared with similar porosity features (Ni-C) and to Ni nanoparticles deposited on a commercial carbon (Ni-Cref). The efficiency of these materials was compared for reactions performed both in batch and flow reactors, highlighting the effect of the reactor setup on the stability of the recovered catalysts.", publisher = "Amer Chemical Soc, Washington", journal = "ACS Sustainable Chemistry and Engineering", title = "Efficiency of Ni Nanoparticles Supported on Hierarchical Porous Nitrogen-Doped Carbon for Hydrogenolysis of Kraft Lignin in Flow and Batch Systems", volume = "5", number = "3", pages = "2415-2420", doi = "10.1021/acssuschemeng.6b02761" }
Lama, S. M.G., Pampel, J., Fellinger, T., Beškoski, V., Slavković-Beškoski, L., Antonietti, M.,& Molinari, V.. (2017). Efficiency of Ni Nanoparticles Supported on Hierarchical Porous Nitrogen-Doped Carbon for Hydrogenolysis of Kraft Lignin in Flow and Batch Systems. in ACS Sustainable Chemistry and Engineering Amer Chemical Soc, Washington., 5(3), 2415-2420. https://doi.org/10.1021/acssuschemeng.6b02761
Lama SM, Pampel J, Fellinger T, Beškoski V, Slavković-Beškoski L, Antonietti M, Molinari V. Efficiency of Ni Nanoparticles Supported on Hierarchical Porous Nitrogen-Doped Carbon for Hydrogenolysis of Kraft Lignin in Flow and Batch Systems. in ACS Sustainable Chemistry and Engineering. 2017;5(3):2415-2420. doi:10.1021/acssuschemeng.6b02761 .
Lama, Sandy M.G., Pampel, Jonas, Fellinger, Tim-Patrick, Beškoski, Vladimir, Slavković-Beškoski, Latinka, Antonietti, Markus, Molinari, Valerio, "Efficiency of Ni Nanoparticles Supported on Hierarchical Porous Nitrogen-Doped Carbon for Hydrogenolysis of Kraft Lignin in Flow and Batch Systems" in ACS Sustainable Chemistry and Engineering, 5, no. 3 (2017):2415-2420, https://doi.org/10.1021/acssuschemeng.6b02761 . .