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Geochemical distribution of selected elements in flotation tailings and soils/sediments from the dam spill at the abandoned antimony mine Stolice, Serbia

Authorized Users Only
2020
Authors
Ranđelović, Dragana
Mutić, Jelena
Marjanović, Prvoslav
Đorđević, Tamara
Kašanin-Grubin, Milica
Article (Published version)
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Abstract
Materials held within mine tailings pose a serious risk to the environment in cases of tailings dam failure. Collapse of the tailing dam at the Stolice antimony mine in West Serbia caused a spilling of tailing slurry into the nearby river watersheds. Medium-term effects of As, Pb, Sb, Zn, and Cd from the tailings material that remained in the flooded zone 3 years after the initial exposure were evaluated. Mobility of these elements was determined by analyzing their distribution between exchangeable, reducible, oxidizable, and residual phases. Results indicate that Fe-Mn oxides represent important sinks for As, Cd, Pb, and Sb. Multivariate statistical analysis revealed that concentrations of the analyzed elements were related to sand-sized fractions, as they tended to adsorb or co-precipitate as coatings on larger particles (particularly feldspar and quartz) upon the change of redox conditions. Assessment of the most relevant physico-chemical factors, metal(loid) concentration, and mobi...lity can be used as tool to characterize the degree of contamination of impacted sites. Percentage of sand-sized particles, content of investigated metal(loid)s, and their amount in the reducible fractions are factors determining the best remediation techniques for the area impacted by tailing spill.

Keywords:
Flotation tailings spill / Metal(oid)s / Risk assessment / Soil
Source:
Environmental Science and Pollution Research, 2020, 27, 6, 6253-6268
Publisher:
  • Springer
Funding / projects:
  • Application of advanced oxidation processes and nanostructured oxide materials for the removal of pollutants from the environment, development and optimisation of instrumental techniques for efficiency monitoring (RS-172030)
  • Magmatism and geodynamics of the Balkan Peninsula from Mesozoic to present day: significance for the formation of metallic and non-metallic mineral deposits (RS-176016)
  • Geochemical investigations of sedimentary rocks - fossil fuels and environmental pollutants (RS-176006)
Note:
  • Supplementary material: http://cherry.chem.bg.ac.rs/handle/123456789/3967

DOI: 10.1007/s11356-019-07348-4

ISSN: 0944-1344

WoS: 000503669600003

Scopus: 2-s2.0-85077063885
[ Google Scholar ]
6
3
URI
https://cherry.chem.bg.ac.rs/handle/123456789/3966
Collections
  • Publikacije / Publications
Institution/Community
Hemijski fakultet / Faculty of Chemistry
TY  - JOUR
AU  - Ranđelović, Dragana
AU  - Mutić, Jelena
AU  - Marjanović, Prvoslav
AU  - Đorđević, Tamara
AU  - Kašanin-Grubin, Milica
PY  - 2020
UR  - https://cherry.chem.bg.ac.rs/handle/123456789/3966
AB  - Materials held within mine tailings pose a serious risk to the environment in cases of tailings dam failure. Collapse of the tailing dam at the Stolice antimony mine in West Serbia caused a spilling of tailing slurry into the nearby river watersheds. Medium-term effects of As, Pb, Sb, Zn, and Cd from the tailings material that remained in the flooded zone 3 years after the initial exposure were evaluated. Mobility of these elements was determined by analyzing their distribution between exchangeable, reducible, oxidizable, and residual phases. Results indicate that Fe-Mn oxides represent important sinks for As, Cd, Pb, and Sb. Multivariate statistical analysis revealed that concentrations of the analyzed elements were related to sand-sized fractions, as they tended to adsorb or co-precipitate as coatings on larger particles (particularly feldspar and quartz) upon the change of redox conditions. Assessment of the most relevant physico-chemical factors, metal(loid) concentration, and mobility can be used as tool to characterize the degree of contamination of impacted sites. Percentage of sand-sized particles, content of investigated metal(loid)s, and their amount in the reducible fractions are factors determining the best remediation techniques for the area impacted by tailing spill.
PB  - Springer
T2  - Environmental Science and Pollution Research
T1  - Geochemical distribution of selected elements in flotation tailings and soils/sediments from the dam spill at the abandoned antimony mine Stolice, Serbia
VL  - 27
IS  - 6
SP  - 6253
EP  - 6268
DO  - 10.1007/s11356-019-07348-4
ER  - 
@article{
author = "Ranđelović, Dragana and Mutić, Jelena and Marjanović, Prvoslav and Đorđević, Tamara and Kašanin-Grubin, Milica",
year = "2020",
abstract = "Materials held within mine tailings pose a serious risk to the environment in cases of tailings dam failure. Collapse of the tailing dam at the Stolice antimony mine in West Serbia caused a spilling of tailing slurry into the nearby river watersheds. Medium-term effects of As, Pb, Sb, Zn, and Cd from the tailings material that remained in the flooded zone 3 years after the initial exposure were evaluated. Mobility of these elements was determined by analyzing their distribution between exchangeable, reducible, oxidizable, and residual phases. Results indicate that Fe-Mn oxides represent important sinks for As, Cd, Pb, and Sb. Multivariate statistical analysis revealed that concentrations of the analyzed elements were related to sand-sized fractions, as they tended to adsorb or co-precipitate as coatings on larger particles (particularly feldspar and quartz) upon the change of redox conditions. Assessment of the most relevant physico-chemical factors, metal(loid) concentration, and mobility can be used as tool to characterize the degree of contamination of impacted sites. Percentage of sand-sized particles, content of investigated metal(loid)s, and their amount in the reducible fractions are factors determining the best remediation techniques for the area impacted by tailing spill.",
publisher = "Springer",
journal = "Environmental Science and Pollution Research",
title = "Geochemical distribution of selected elements in flotation tailings and soils/sediments from the dam spill at the abandoned antimony mine Stolice, Serbia",
volume = "27",
number = "6",
pages = "6253-6268",
doi = "10.1007/s11356-019-07348-4"
}
Ranđelović, D., Mutić, J., Marjanović, P., Đorđević, T.,& Kašanin-Grubin, M.. (2020). Geochemical distribution of selected elements in flotation tailings and soils/sediments from the dam spill at the abandoned antimony mine Stolice, Serbia. in Environmental Science and Pollution Research
Springer., 27(6), 6253-6268.
https://doi.org/10.1007/s11356-019-07348-4
Ranđelović D, Mutić J, Marjanović P, Đorđević T, Kašanin-Grubin M. Geochemical distribution of selected elements in flotation tailings and soils/sediments from the dam spill at the abandoned antimony mine Stolice, Serbia. in Environmental Science and Pollution Research. 2020;27(6):6253-6268.
doi:10.1007/s11356-019-07348-4 .
Ranđelović, Dragana, Mutić, Jelena, Marjanović, Prvoslav, Đorđević, Tamara, Kašanin-Grubin, Milica, "Geochemical distribution of selected elements in flotation tailings and soils/sediments from the dam spill at the abandoned antimony mine Stolice, Serbia" in Environmental Science and Pollution Research, 27, no. 6 (2020):6253-6268,
https://doi.org/10.1007/s11356-019-07348-4 . .

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