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Is a Lead Isotope Ratios in Wine Good Marker for Origin Assessment?

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2021
Is_a_Lead_pub_2021.pdf (2.218Mb)
Authors
Đurđić, Slađana Z.
Stanković, Vesna
Ražić, Slavica
Mutić, Jelena
Article (Published version)
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Abstract
Lead isotope ratio pattern (206Pb/207Pb, 208Pb/206Pb, 206Pb/204Pb, 207Pb/204Pb, and 208Pb/204Pb) was analyzed in 59 samples of Serbian wine, from four geographical regions. By utilization of powerful inductively coupled plasma mass spectrometry (ICP-QMS), lead isotope ratios were used as unique “fingerprint”, when combined with multivariate methods of analysis (Principal Component Analysis), provided information on the geographical origin of wine. In validation of ICP- QMS method and quantitative analysis, the certified reference material NIST SRM 981 was employed to test the mass-bias correction and thallium isotopes 203Tl and 205Tl (NIST SRM 997) as an internal standard. The obtained results were discussed in correlation with the corresponding values of LIRs of different European and Australian wines. In addition, the impact of anthropogenic Pb from different sources on the total Pb isotopic composition in Serbian wines was analyzed too. On the other side, the obtained values of Pb c...ontent were compared with the applicable health safety standards, according to the International Code of Oenological Practices.

Keywords:
ICP-QMS / Serbian wines / principal component analysis / geographical origin / lead isotopes
Source:
Frontiers in Chemistry, 2021, 9, 842-
Publisher:
  • Frontiers Media
Funding / projects:
  • Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 200168 (University of Belgrade, Faculty of Chemistry) (RS-200168)
  • Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 200161 (University of Belgrade, Faculty of Pharmacy) (RS-200161)
Note:
  • Supplementary material: https://cherry.chem.bg.ac.rs/handle/123456789/4749
Related info:
  • Referenced by
    https://cherry.chem.bg.ac.rs/handle/123456789/4749

DOI: 10.3389/fchem.2021.746695

ISSN: 2296-2646

WoS: 000717096800001

Scopus: 2-s2.0-85117250343
[ Google Scholar ]
URI
https://cherry.chem.bg.ac.rs/handle/123456789/4748
Collections
  • Publikacije
Institution/Community
Hemijski fakultet
TY  - JOUR
AU  - Đurđić, Slađana Z.
AU  - Stanković, Vesna
AU  - Ražić, Slavica
AU  - Mutić, Jelena
PY  - 2021
UR  - https://cherry.chem.bg.ac.rs/handle/123456789/4748
AB  - Lead isotope ratio pattern (206Pb/207Pb, 208Pb/206Pb, 206Pb/204Pb, 207Pb/204Pb, and 208Pb/204Pb) was analyzed in 59 samples of Serbian wine, from four geographical regions. By utilization of powerful inductively coupled plasma mass spectrometry (ICP-QMS), lead isotope ratios were used as unique “fingerprint”, when combined with multivariate methods of analysis (Principal Component Analysis), provided information on the geographical origin of wine. In validation of ICP- QMS method and quantitative analysis, the certified reference material NIST SRM 981 was employed to test the mass-bias correction and thallium isotopes 203Tl and 205Tl (NIST SRM 997) as an internal standard. The obtained results were discussed in correlation with the corresponding values of LIRs of different European and Australian wines. In addition, the impact of anthropogenic Pb from different sources on the total Pb isotopic composition in Serbian wines was analyzed too. On the other side, the obtained values of Pb content were compared with the applicable health safety standards, according to the International Code of Oenological Practices.
PB  - Frontiers Media
T2  - Frontiers in Chemistry
T1  - Is a Lead Isotope Ratios in Wine Good Marker for Origin Assessment?
VL  - 9
SP  - 842
DO  - 10.3389/fchem.2021.746695
ER  - 
@article{
author = "Đurđić, Slađana Z. and Stanković, Vesna and Ražić, Slavica and Mutić, Jelena",
year = "2021",
abstract = "Lead isotope ratio pattern (206Pb/207Pb, 208Pb/206Pb, 206Pb/204Pb, 207Pb/204Pb, and 208Pb/204Pb) was analyzed in 59 samples of Serbian wine, from four geographical regions. By utilization of powerful inductively coupled plasma mass spectrometry (ICP-QMS), lead isotope ratios were used as unique “fingerprint”, when combined with multivariate methods of analysis (Principal Component Analysis), provided information on the geographical origin of wine. In validation of ICP- QMS method and quantitative analysis, the certified reference material NIST SRM 981 was employed to test the mass-bias correction and thallium isotopes 203Tl and 205Tl (NIST SRM 997) as an internal standard. The obtained results were discussed in correlation with the corresponding values of LIRs of different European and Australian wines. In addition, the impact of anthropogenic Pb from different sources on the total Pb isotopic composition in Serbian wines was analyzed too. On the other side, the obtained values of Pb content were compared with the applicable health safety standards, according to the International Code of Oenological Practices.",
publisher = "Frontiers Media",
journal = "Frontiers in Chemistry",
title = "Is a Lead Isotope Ratios in Wine Good Marker for Origin Assessment?",
volume = "9",
pages = "842",
doi = "10.3389/fchem.2021.746695"
}
Đurđić, S. Z., Stanković, V., Ražić, S.,& Mutić, J.. (2021). Is a Lead Isotope Ratios in Wine Good Marker for Origin Assessment?. in Frontiers in Chemistry
Frontiers Media., 9, 842.
https://doi.org/10.3389/fchem.2021.746695
Đurđić SZ, Stanković V, Ražić S, Mutić J. Is a Lead Isotope Ratios in Wine Good Marker for Origin Assessment?. in Frontiers in Chemistry. 2021;9:842.
doi:10.3389/fchem.2021.746695 .
Đurđić, Slađana Z., Stanković, Vesna, Ražić, Slavica, Mutić, Jelena, "Is a Lead Isotope Ratios in Wine Good Marker for Origin Assessment?" in Frontiers in Chemistry, 9 (2021):842,
https://doi.org/10.3389/fchem.2021.746695 . .

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