Comparative life cycle assessment of Ni-based catalyst synthesis processes
Само за регистроване кориснике
2017
Чланак у часопису (Објављена верзија)
Метаподаци
Приказ свих података о документуАпстракт
Ni-based catalysts supported on ceramics are particularly suitable for industrial applications, for instance reforming of hydrocarbons to produce synthesis gas or hydrogen and production of carbon nanofibers. Conventional synthesis processes for all metal/ceramic catalysts are impregnation, precipitation, coprecipitation and others. The authors have previously developed a novel process for the synthesis of Ni-based catalysts supported on reticulated ceramic foams, including impregnation of foams with ultrasonically generated aerosols of dissolved metal chlorides. By using appropriate multi-criteria analysis methods, the authors concluded that the novel process for the synthesis of Ni-based catalysts was superior in terms of economic and technological aspects. The aim of this research was to compare the novel synthesis processes for a Ni-Pd/Al2O3 catalyst and for other Ni-based catalysts by performing life cycle assessment and evaluating the environmental impacts of each synthesis proce...ss. Characterisation results
showed that the dominant environmental impact results from production of palladium (II) chloride for the Ni-Pd/Al2O3 catalyst synthesis process, while the other catalyst synthesis process had large environmental impacts associated with high energy consumption. The final outcome, obtained from comparison of normalisation results, indicates that the novel Ni-Pd/Al2O3 catalyst synthesis process had the smallest environmental impact.
Кључне речи:
Novel synthesis process / Life cycle assessment / Ni-based catalystИзвор:
Journal of Cleaner Production, 2017, 162, 7-15Издавач:
- Elsevier
Финансирање / пројекти:
- Иновативна синергија нус-продуката, минимизације отпада и чистије производње у металургији (RS-34033)
DOI: 10.1016/j.jclepro.2017.06.012
ISSN: 0959-6526
WoS: 000407185500002
Scopus: 2-s2.0-85024099298
Колекције
Институција/група
Inovacioni centar / Innovation CentreTY - JOUR AU - Agarski, Boris AU - Nikolić, Vesna AU - Kamberović, Željko AU - Anđić, Zoran AU - Kosec, Borut AU - Budak, Igor PY - 2017 UR - http://cherry.chem.bg.ac.rs/handle/123456789/5050 AB - Ni-based catalysts supported on ceramics are particularly suitable for industrial applications, for instance reforming of hydrocarbons to produce synthesis gas or hydrogen and production of carbon nanofibers. Conventional synthesis processes for all metal/ceramic catalysts are impregnation, precipitation, coprecipitation and others. The authors have previously developed a novel process for the synthesis of Ni-based catalysts supported on reticulated ceramic foams, including impregnation of foams with ultrasonically generated aerosols of dissolved metal chlorides. By using appropriate multi-criteria analysis methods, the authors concluded that the novel process for the synthesis of Ni-based catalysts was superior in terms of economic and technological aspects. The aim of this research was to compare the novel synthesis processes for a Ni-Pd/Al2O3 catalyst and for other Ni-based catalysts by performing life cycle assessment and evaluating the environmental impacts of each synthesis process. Characterisation results showed that the dominant environmental impact results from production of palladium (II) chloride for the Ni-Pd/Al2O3 catalyst synthesis process, while the other catalyst synthesis process had large environmental impacts associated with high energy consumption. The final outcome, obtained from comparison of normalisation results, indicates that the novel Ni-Pd/Al2O3 catalyst synthesis process had the smallest environmental impact. PB - Elsevier T2 - Journal of Cleaner Production T1 - Comparative life cycle assessment of Ni-based catalyst synthesis processes VL - 162 SP - 7 EP - 15 DO - 10.1016/j.jclepro.2017.06.012 ER -
@article{ author = "Agarski, Boris and Nikolić, Vesna and Kamberović, Željko and Anđić, Zoran and Kosec, Borut and Budak, Igor", year = "2017", abstract = "Ni-based catalysts supported on ceramics are particularly suitable for industrial applications, for instance reforming of hydrocarbons to produce synthesis gas or hydrogen and production of carbon nanofibers. Conventional synthesis processes for all metal/ceramic catalysts are impregnation, precipitation, coprecipitation and others. The authors have previously developed a novel process for the synthesis of Ni-based catalysts supported on reticulated ceramic foams, including impregnation of foams with ultrasonically generated aerosols of dissolved metal chlorides. By using appropriate multi-criteria analysis methods, the authors concluded that the novel process for the synthesis of Ni-based catalysts was superior in terms of economic and technological aspects. The aim of this research was to compare the novel synthesis processes for a Ni-Pd/Al2O3 catalyst and for other Ni-based catalysts by performing life cycle assessment and evaluating the environmental impacts of each synthesis process. Characterisation results showed that the dominant environmental impact results from production of palladium (II) chloride for the Ni-Pd/Al2O3 catalyst synthesis process, while the other catalyst synthesis process had large environmental impacts associated with high energy consumption. The final outcome, obtained from comparison of normalisation results, indicates that the novel Ni-Pd/Al2O3 catalyst synthesis process had the smallest environmental impact.", publisher = "Elsevier", journal = "Journal of Cleaner Production", title = "Comparative life cycle assessment of Ni-based catalyst synthesis processes", volume = "162", pages = "7-15", doi = "10.1016/j.jclepro.2017.06.012" }
Agarski, B., Nikolić, V., Kamberović, Ž., Anđić, Z., Kosec, B.,& Budak, I.. (2017). Comparative life cycle assessment of Ni-based catalyst synthesis processes. in Journal of Cleaner Production Elsevier., 162, 7-15. https://doi.org/10.1016/j.jclepro.2017.06.012
Agarski B, Nikolić V, Kamberović Ž, Anđić Z, Kosec B, Budak I. Comparative life cycle assessment of Ni-based catalyst synthesis processes. in Journal of Cleaner Production. 2017;162:7-15. doi:10.1016/j.jclepro.2017.06.012 .
Agarski, Boris, Nikolić, Vesna, Kamberović, Željko, Anđić, Zoran, Kosec, Borut, Budak, Igor, "Comparative life cycle assessment of Ni-based catalyst synthesis processes" in Journal of Cleaner Production, 162 (2017):7-15, https://doi.org/10.1016/j.jclepro.2017.06.012 . .